Deadman Wonderland, Casshern Sins, Full Metal Alchemist, Ghost in the Shell, and Eureka 7.

And Kitty got me watching a little bit of Ergo Proxy. =P
 
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Right now I'm watching Accel World when I can.
It teaches us the valuable lesson that fat people can be main characters too.
 
To sum up the entirety of Kaiji in one image:

EaTQH.jpg
 
Now my new favorite anime is offically Shakugan No Shana, spent like a month getting high on that shit
 
Favorites... favorites... I mean, I have too many of them, all varying on genre, appeal, and other random crap, it usually means I end up with a bunch of lists of favorites (i.e. favorite mecha, favorite magical girl series, favorite horror, favorite sc-fi, favorite VN adaptation)

Still, the first that pops to mind is everything done by Junji Ito, especially Uzumaki and Tomie, or most of the stuff done by Fukumoto such as:

 
I thought it was really cool after watching the whole thing but later, I realized how much plotholes and other stuff it is missing.
Meh, I kinda got pissed at the start of each new season due to the fact that they basically bullshit you on the previous seasons ending in some way
 
Cant name them all but top 5 are

1. Gundam Universal century

2. Bakemonogatari

3.Neon Genesis Evangelion

4.Rahxephon

5.Lupin III